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Soothing of Smagol can be cast during the end step, causing your opponent to basically lose a turn while you get to start your turn with the benefits of the Ring

By combining this you can sweep, keep your Commander and then drop all else, at instant speed despite what abilities they have to keep them up

Be'lakor, the Dark Master is the backup Chaos commander, and he's a brutally simple demon tribal commander

While you've likely already missed the prerelease events for Tales of Middle-earth, you can still pick up Prerelease Kits and enjoy the set's sealed format at home

Carsten Kotter wrote a great piece on this topic a couple years ago

A Couple More Cards to Watch In addition to these highly recognizable characters, there are a couple non-creature cards worth cracking open in a Spider-Man play booster